A novel PdNi/Al2O3 catalyst prepared by galvanic deposition for low temperature methane combustion

能源化学(英文) ›› 2013, Vol. 22 ›› Issue (4): 610-616.

A novel PdNi/Al₂O₃ catalyst prepared by galvanic deposition for low temperature methane combustion

Xiqiang Pan^a,b,c, Yibo Zhang^a,b,c, Zhenzhen Miao^a,b,c, Xiangguang Yang^a,b

a. State Key Laboratory of Rare Earth Resource Utilization, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 13002, Jilin, China;
b. Laboratory of Green Chemistry and Process, Changchun Institute of Applied Chemistry, Chinese Academy ofSciences, Changchun 130022, Jilin, China;
c. University of Chinese Academy of Sciences, Beijing 100049, China

收稿日期:2012-05-27 修回日期:2012-08-22 出版日期:2013-07-20 发布日期:2013-07-27
通讯作者: Xiangguang Yang
基金资助:
This work was supported by the National Natural Science Foundation of China (21273221) and the National High Technology Research and Development Program of China (863 Program, 2011AA03A406).

A novel PdNi/Al₂O₃ catalyst prepared by galvanic deposition for low temperature methane combustion

Xiqiang Pan^a,b,c, Yibo Zhang^a,b,c, Zhenzhen Miao^a,b,c, Xiangguang Yang^a,b

a. State Key Laboratory of Rare Earth Resource Utilization, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 13002, Jilin, China;
b. Laboratory of Green Chemistry and Process, Changchun Institute of Applied Chemistry, Chinese Academy ofSciences, Changchun 130022, Jilin, China;
c. University of Chinese Academy of Sciences, Beijing 100049, China

Received:2012-05-27 Revised:2012-08-22 Online:2013-07-20 Published:2013-07-27
Supported by:
This work was supported by the National Natural Science Foundation of China (21273221) and the National High Technology Research and Development Program of China (863 Program, 2011AA03A406).

摘要/Abstract

摘要： Galvanic deposition method was used to prepare the Pd/Ni-Al₂O₃-GD catalyst for the combustion of methane under lean conditions. The new catalyst and compared catalysts (Pd/Al₂O₃-IW, Pd-Ni/Al₂O₃-IW, Pd/Ni-Al₂O₃-IW) prepared by incipient wetness impregnation were characterized by N₂-physisorption, XRD and TEM to clarify particle size and size distribution of palladium species. Combined O₂-TPD and XPS results with the catalytic data, it shows that the surface palladium species with low valence exhibits better combustion performance due to their stronger interaction with support. The results indicate that the galvanic deposition method is an effective route to prepare efficient catalyst for methane combustion, and it also provides useful information for improving the present commercial catalyst.

关键词: methane, catalytic combustion, palladium, Pd/Al₂O₃, galvanic replace reaction

Abstract: Galvanic deposition method was used to prepare the Pd/Ni-Al₂O₃-GD catalyst for the combustion of methane under lean conditions. The new catalyst and compared catalysts (Pd/Al₂O₃-IW, Pd-Ni/Al₂O₃-IW, Pd/Ni-Al₂O₃-IW) prepared by incipient wetness impregnation were characterized by N₂-physisorption, XRD and TEM to clarify particle size and size distribution of palladium species. Combined O₂-TPD and XPS results with the catalytic data, it shows that the surface palladium species with low valence exhibits better combustion performance due to their stronger interaction with support. The results indicate that the galvanic deposition method is an effective route to prepare efficient catalyst for methane combustion, and it also provides useful information for improving the present commercial catalyst.

Key words: methane, catalytic combustion, palladium, Pd/Al₂O₃, galvanic replace reaction

Xiqiang Pan, Yibo Zhang, Zhenzhen Miao, Xiangguang Yang. A novel PdNi/Al₂O₃ catalyst prepared by galvanic deposition for low temperature methane combustion[J]. 能源化学(英文), 2013, 22(4): 610-616.

Xiqiang Pan, Yibo Zhang, Zhenzhen Miao, Xiangguang Yang. A novel PdNi/Al₂O₃ catalyst prepared by galvanic deposition for low temperature methane combustion[J]. Journal of Energy Chemistry, 2013, 22(4): 610-616.

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A novel PdNi/Al₂O₃ catalyst prepared by galvanic deposition for low temperature methane combustion

A novel PdNi/Al₂O₃ catalyst prepared by galvanic deposition for low temperature methane combustion

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