Advances in efficient electrocatalysts based on layered double hydroxides and their derivatives

doi:10.1016/j.jechem.2017.09.015

能源化学(英文) ›› 2017, Vol. 26 ›› Issue (6): 1094-1106.DOI: 10.1016/j.jechem.2017.09.015

Advances in efficient electrocatalysts based on layered double hydroxides and their derivatives

Lei Zhou, Mingfei Shao, Min Wei, Xue Duan

State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing 100029, China

收稿日期:2017-09-02 修回日期:2017-09-15 出版日期:2017-11-15 发布日期:2017-11-24
通讯作者: Mingfei Shao,E-mail address:shaomf@mail.buct.edu.cn
作者简介:Lei Zhou received her Bachelor's degree in 2013 from Beijing University of Chemical Technology;Lei Zhou received her Bachelor's degree in 2013 from Beijing University of Chemical Technology;Min Wei obtained her B.Eng. degree in 1995 and M.Eng. degree in 1998 from Beijing University of Chemical Technology (BUCT);Xue Duan was elected as an Academician of the Chinese Academy of Sciences in 2007.
基金资助:
This work was supported by the National Natural Science Foundation of China (Nos. U1462118; 21601011), the 973 Program (Grant No. 2014CB932102) and the Fundamental Research Funds for the Central Universities (buctrc201506; PYCC1704).

Advances in efficient electrocatalysts based on layered double hydroxides and their derivatives

Lei Zhou, Mingfei Shao, Min Wei, Xue Duan

State Key Laboratory of Chemical Resource Engineering, Beijing University of Chemical Technology, Beijing 100029, China

Received:2017-09-02 Revised:2017-09-15 Online:2017-11-15 Published:2017-11-24
Contact: Mingfei Shao,E-mail address:shaomf@mail.buct.edu.cn
About author:Lei Zhou received her Bachelor's degree in 2013 from Beijing University of Chemical Technology;Lei Zhou received her Bachelor's degree in 2013 from Beijing University of Chemical Technology;Min Wei obtained her B.Eng. degree in 1995 and M.Eng. degree in 1998 from Beijing University of Chemical Technology (BUCT);Xue Duan was elected as an Academician of the Chinese Academy of Sciences in 2007.
Supported by:
This work was supported by the National Natural Science Foundation of China (Nos. U1462118; 21601011), the 973 Program (Grant No. 2014CB932102) and the Fundamental Research Funds for the Central Universities (buctrc201506; PYCC1704).

摘要/Abstract

摘要： The explore and development of electrocatalysts have gained significant attention due to their indispensable status in energy storage and conversion systems, such as fuel cells, metal-air batteries and solar water splitting cells. Layered double hydroxides (LDHs) and their derivatives (e.g., transition metal alloys, oxides, sulfides, nitrides and phosphides) have been adopted as catalysts for various electrochemical reactions, such as oxygen reduction, oxygen evolution, hydrogen evolution, and CO₂ reduction, which show excellent activity and remarkable durability in electrocatalytic process. In this review, the synthesis strategies, structural characters and electrochemical performances for the LDHs and their derivatives are described. In addition, we also discussed the effect of electronic and geometry structures to their electrocatalytic activity. The further development of high-performance electrocatalysts based on LDHs and their derivatives is covered by both a short summary and future outlook from the viewpoint of the material design and practical application.

关键词: Layered double hydroxide, Derivatives, Electrocatalysis, Oxygen reduction, Water splitting, CO₂ reduction, Electronic structure, Hierarchical structure, Metal-air battery, Fuel cell

Abstract: The explore and development of electrocatalysts have gained significant attention due to their indispensable status in energy storage and conversion systems, such as fuel cells, metal-air batteries and solar water splitting cells. Layered double hydroxides (LDHs) and their derivatives (e.g., transition metal alloys, oxides, sulfides, nitrides and phosphides) have been adopted as catalysts for various electrochemical reactions, such as oxygen reduction, oxygen evolution, hydrogen evolution, and CO₂ reduction, which show excellent activity and remarkable durability in electrocatalytic process. In this review, the synthesis strategies, structural characters and electrochemical performances for the LDHs and their derivatives are described. In addition, we also discussed the effect of electronic and geometry structures to their electrocatalytic activity. The further development of high-performance electrocatalysts based on LDHs and their derivatives is covered by both a short summary and future outlook from the viewpoint of the material design and practical application.

Key words: Layered double hydroxide, Derivatives, Electrocatalysis, Oxygen reduction, Water splitting, CO₂ reduction, Electronic structure, Hierarchical structure, Metal-air battery, Fuel cell

Lei Zhou, Mingfei Shao, Min Wei, Xue Duan. Advances in efficient electrocatalysts based on layered double hydroxides and their derivatives[J]. 能源化学(英文), 2017, 26(6): 1094-1106.

Lei Zhou, Mingfei Shao, Min Wei, Xue Duan. Advances in efficient electrocatalysts based on layered double hydroxides and their derivatives[J]. Journal of Energy Chemistry, 2017, 26(6): 1094-1106.

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Advances in efficient electrocatalysts based on layered double hydroxides and their derivatives

Advances in efficient electrocatalysts based on layered double hydroxides and their derivatives

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