The roles of graphene in advanced Li-ion hybrid supercapacitors

doi:10.1016/j.jechem.2017.11.020

能源化学(英文) ›› 2018, Vol. 27 ›› Issue (1): 43-56.DOI: 10.1016/j.jechem.2017.11.020

The roles of graphene in advanced Li-ion hybrid supercapacitors

Junwei Lang^a,b, Xu Zhang^a, Bao Liu^a, Rutao Wang^a, Jiangtao Chen^a, Xingbin Yan^a

a Laboratory of Clean Energy Chemistry and Materials, State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Lanzhou 730000, Gansu, China;
b Qingdao Center of Resource Chemistry & New Materials, Qingdao 266071, Shandong, China

收稿日期:2017-10-17 修回日期:2017-11-15 出版日期:2018-01-15 发布日期:2018-01-13
通讯作者: Xingbin Yan
作者简介:Junwei Lang received her Ph.D. degree at Lanzhou University of Technology in 2010;Xu Zhang completed his BS and MS degree in 2009 and 2013 at Lanzhou Jiaotong University, respectively;Bao Liu received his BS degree at Jiangxi University of Science and technology in 2015;Rutao Wang received his Ph.D. Degree in Materials Science in 2015 at LICP, CAS.
基金资助:
This work was supported by the National Nature Science Foundations of China (Grant No. 21673263, 21573265), the Independent Innovation Plan Foundations of Qingdao City of China (Grant No. 16-5-1-42-jch) and the western Young Scholars Foundations of Chinese Academy of Sciences.

The roles of graphene in advanced Li-ion hybrid supercapacitors

Junwei Lang^a,b, Xu Zhang^a, Bao Liu^a, Rutao Wang^a, Jiangtao Chen^a, Xingbin Yan^a

a Laboratory of Clean Energy Chemistry and Materials, State Key Laboratory of Solid Lubrication, Lanzhou Institute of Chemical Physics, Lanzhou 730000, Gansu, China;
b Qingdao Center of Resource Chemistry & New Materials, Qingdao 266071, Shandong, China

Received:2017-10-17 Revised:2017-11-15 Online:2018-01-15 Published:2018-01-13
Contact: Xingbin Yan
Supported by:
This work was supported by the National Nature Science Foundations of China (Grant No. 21673263, 21573265), the Independent Innovation Plan Foundations of Qingdao City of China (Grant No. 16-5-1-42-jch) and the western Young Scholars Foundations of Chinese Academy of Sciences.

摘要/Abstract

摘要： Lithium-ion hybrid supercapacitors (LIHSs), also called Li-ion capacitors, are electrochemical energy storage devices that combining the advantages of high power density of supercapacitor and high energy density of Li-ion battery. However, high power density and long cycle life are still challenges for the current LIHSs due to the imbalance of charge-storage capacity and electrode kinetics between capacitor-type cathode and battery-type anode. Therefore, great efforts have been made on designing novel cathode materials with high storage capacity and anode material with enhanced kinetic behavior for LIHSs. With unique two-dimensional form and numerous appealing properties, for the past several years, the rational designed graphene and its composites materials exhibit greatly improved electrochemical performance as cathode or anode for LIHSs. Here, we summarized and discussed the latest advances of the stateof-art graphene-based materials for LIHSs applications. The major roles of graphene are highlighted as (1) a superior active material, (2) ultrathin 2D flexible support to remedy the sluggish reaction of the metal compound anode, and (3) good 2D building blocks for constructing macroscopic 3D porous carbon/graphene hybrids. In addition, some high performance aqueous LIHSs using graphene as electrode were also summarized. Finally, the perspectives and challenges are also proposed for further development of more advanced graphene-based LIHSs.

关键词: Graphene, Li-ion hybrid supercapacitors, Supercapacitor, Lithium ion batteries, Carbon materials, Metal oxide, Nanocomposites

Abstract: Lithium-ion hybrid supercapacitors (LIHSs), also called Li-ion capacitors, are electrochemical energy storage devices that combining the advantages of high power density of supercapacitor and high energy density of Li-ion battery. However, high power density and long cycle life are still challenges for the current LIHSs due to the imbalance of charge-storage capacity and electrode kinetics between capacitor-type cathode and battery-type anode. Therefore, great efforts have been made on designing novel cathode materials with high storage capacity and anode material with enhanced kinetic behavior for LIHSs. With unique two-dimensional form and numerous appealing properties, for the past several years, the rational designed graphene and its composites materials exhibit greatly improved electrochemical performance as cathode or anode for LIHSs. Here, we summarized and discussed the latest advances of the stateof-art graphene-based materials for LIHSs applications. The major roles of graphene are highlighted as (1) a superior active material, (2) ultrathin 2D flexible support to remedy the sluggish reaction of the metal compound anode, and (3) good 2D building blocks for constructing macroscopic 3D porous carbon/graphene hybrids. In addition, some high performance aqueous LIHSs using graphene as electrode were also summarized. Finally, the perspectives and challenges are also proposed for further development of more advanced graphene-based LIHSs.

Key words: Graphene, Li-ion hybrid supercapacitors, Supercapacitor, Lithium ion batteries, Carbon materials, Metal oxide, Nanocomposites

Junwei Lang, Xu Zhang, Bao Liu, Rutao Wang, Jiangtao Chen, Xingbin Yan. The roles of graphene in advanced Li-ion hybrid supercapacitors[J]. 能源化学(英文), 2018, 27(1): 43-56.

Junwei Lang, Xu Zhang, Bao Liu, Rutao Wang, Jiangtao Chen, Xingbin Yan. The roles of graphene in advanced Li-ion hybrid supercapacitors[J]. Journal of Energy Chemistry, 2018, 27(1): 43-56.

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The roles of graphene in advanced Li-ion hybrid supercapacitors

The roles of graphene in advanced Li-ion hybrid supercapacitors

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