Recent advances of graphene-based materials for high-performance and new-concept supercapacitors

doi:10.1016/j.jechem.2017.09.034

能源化学(英文) ›› 2018, Vol. 27 ›› Issue (1): 25-42.DOI: 10.1016/j.jechem.2017.09.034

Recent advances of graphene-based materials for high-performance and new-concept supercapacitors

Xiaoyu Shi^a,b,c, Shuanghao Zheng^a,b,d, Zhong-Shuai Wu^a, Xinhe Bao^a,b

a Dalian National Laboratory for Clean Energy, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457 Zhongshan Road, Dalian 116023, Liaoning, China;
b State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457 Zhongshan Road, Dalian 116023, Liaoning, China;
c Department of Chemical Physics, University of Science and Technology of China, 96 JinZhai Road, Hefei 230026, Anhui, China;
d University of Chinese Academy of Sciences, 19 A Yuquan Road, Beijing 100049, China

收稿日期:2017-09-20 修回日期:2017-09-29 出版日期:2018-01-15 发布日期:2018-01-13
通讯作者: Zhong-Shuai Wu
作者简介:Xiaoyu Shi received his B.S. degree from Nankai University in 2015;Shuanghao Zheng is now pursuing the Ph.D. degree from Dalian National Laboratory for Clean Energy, DICP, CAS, under the supervision of Prof;Zhong-Shuai Wu received his Ph.D. in materials science from Institute of Metal Research, CAS in 2011, and worked as a postdoctor at Max-Planck Institute for Polymer Research in 2011-2015.
基金资助:
This work was financially supported by the National Natural Science Foundation of China (Grant 51572259), National Key R&D Program of China (Grant 2016YBF0100100 and 2016YFA0200200), Natural Science Foundation of Liaoning Province (Grant 201602737), Thousand Youth Talents Plan of China, DICP (DICP ZZBS201708), and Exploratory Research Projects of Shaanxi Yanchang Petroleum (Group) CO., LTD & DICP.

Recent advances of graphene-based materials for high-performance and new-concept supercapacitors

Xiaoyu Shi^a,b,c, Shuanghao Zheng^a,b,d, Zhong-Shuai Wu^a, Xinhe Bao^a,b

a Dalian National Laboratory for Clean Energy, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457 Zhongshan Road, Dalian 116023, Liaoning, China;
b State Key Laboratory of Catalysis, Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457 Zhongshan Road, Dalian 116023, Liaoning, China;
c Department of Chemical Physics, University of Science and Technology of China, 96 JinZhai Road, Hefei 230026, Anhui, China;
d University of Chinese Academy of Sciences, 19 A Yuquan Road, Beijing 100049, China

Received:2017-09-20 Revised:2017-09-29 Online:2018-01-15 Published:2018-01-13
Contact: Zhong-Shuai Wu
Supported by:
This work was financially supported by the National Natural Science Foundation of China (Grant 51572259), National Key R&D Program of China (Grant 2016YBF0100100 and 2016YFA0200200), Natural Science Foundation of Liaoning Province (Grant 201602737), Thousand Youth Talents Plan of China, DICP (DICP ZZBS201708), and Exploratory Research Projects of Shaanxi Yanchang Petroleum (Group) CO., LTD & DICP.

摘要/Abstract

摘要： Supercapacitors, with ultrahigh power density, superior rate capability, long-term cyclability, and exceptional safety, are regarded as one highly competitive candidate of electrochemical energy storage devices, filling the gap between batteries and conventional capacitors. Despite of tremendous effort, elaborated screening of high-performance electrode materials, e.g., graphene, is still intensively required. In this review, we describe the most recent progress in the research and development of graphene-based materials for high-performance and new-concept supercapacitors for the targeted applications in next-generation and smart electronics. First, the design and fabrication of high-performance supercapacitors, including electrical double layer capacitors, pseudocapacitors and hybrid supercapacitors, were summarized in term of the charge storage mechanism. Second, new-concept supercapacitors with multiple functionalities of high-voltage, fiber-shape, microscale and shape-diversity in order to fulfill the requirements of future electronics are reviewed. Accordingly, special emphasis is given to the structure-dependent-performance effects of pores, hybridization, dimensionalities of graphene-based materials on performance of supercapacitors, and tremendous potential of graphene-based planar micro-supercapacitors for the direct seamlessly integration with versatile micro-electronics. Finally, perspectives and challenges of graphene-based supercapacitors are briefly discussed.

关键词: Graphene, Supercapacitors, Energy storage, High performance, New concept

Abstract: Supercapacitors, with ultrahigh power density, superior rate capability, long-term cyclability, and exceptional safety, are regarded as one highly competitive candidate of electrochemical energy storage devices, filling the gap between batteries and conventional capacitors. Despite of tremendous effort, elaborated screening of high-performance electrode materials, e.g., graphene, is still intensively required. In this review, we describe the most recent progress in the research and development of graphene-based materials for high-performance and new-concept supercapacitors for the targeted applications in next-generation and smart electronics. First, the design and fabrication of high-performance supercapacitors, including electrical double layer capacitors, pseudocapacitors and hybrid supercapacitors, were summarized in term of the charge storage mechanism. Second, new-concept supercapacitors with multiple functionalities of high-voltage, fiber-shape, microscale and shape-diversity in order to fulfill the requirements of future electronics are reviewed. Accordingly, special emphasis is given to the structure-dependent-performance effects of pores, hybridization, dimensionalities of graphene-based materials on performance of supercapacitors, and tremendous potential of graphene-based planar micro-supercapacitors for the direct seamlessly integration with versatile micro-electronics. Finally, perspectives and challenges of graphene-based supercapacitors are briefly discussed.

Key words: Graphene, Supercapacitors, Energy storage, High performance, New concept

Xiaoyu Shi, Shuanghao Zheng, Zhong-Shuai Wu, Xinhe Bao. Recent advances of graphene-based materials for high-performance and new-concept supercapacitors[J]. 能源化学(英文), 2018, 27(1): 25-42.

Xiaoyu Shi, Shuanghao Zheng, Zhong-Shuai Wu, Xinhe Bao. Recent advances of graphene-based materials for high-performance and new-concept supercapacitors[J]. Journal of Energy Chemistry, 2018, 27(1): 25-42.

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Recent advances of graphene-based materials for high-performance and new-concept supercapacitors

Recent advances of graphene-based materials for high-performance and new-concept supercapacitors

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