能源化学(英文版)

能源化学(英文) ›› 2018, Vol. 27 ›› Issue (1): 128-145.DOI: 10.1016/j.jechem.2017.11.031

• Preface • 上一篇    下一篇

Two-dimensional nanosheets as building blocks to construct three-dimensional structures for lithium storage

Di Zhang, Shuai Wang, Yang Ma, Shubin Yang   

  1. Key Laboratory of Aerospace Advanced Materials and Performance of Ministry of Education, School of Materials Science & Engineering, Beihang University, Beijing 100191, China
  • 收稿日期:2017-11-22 修回日期:2017-11-27 出版日期:2018-01-15 发布日期:2018-01-13
  • 通讯作者: Shubin Yang
  • 作者简介:Di Zhang received his M.S. degree in Beijing University of Chemical Technology in 2015;Shubin Yang
  • 基金资助:

    This work was financially supported by the National Science Foundation of China (Nos. 51572007 and 51622203), "Recruitment Program of Global Experts"

Two-dimensional nanosheets as building blocks to construct three-dimensional structures for lithium storage

Di Zhang, Shuai Wang, Yang Ma, Shubin Yang   

  1. Key Laboratory of Aerospace Advanced Materials and Performance of Ministry of Education, School of Materials Science & Engineering, Beihang University, Beijing 100191, China
  • Received:2017-11-22 Revised:2017-11-27 Online:2018-01-15 Published:2018-01-13
  • Contact: Shubin Yang
  • Supported by:

    This work was financially supported by the National Science Foundation of China (Nos. 51572007 and 51622203), "Recruitment Program of Global Experts"

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摘要： 2D nanosheets such as graphene, silicene, phosphorene, metal dichalcogenides and MXenes are emerging and promising for lithium storage due to their ultrathin nature and corresponding chemical/physical properties. However, the serious restacking and aggregation of the 2D nanosheets are still hampering their applications. To circumvent the issues of 2D nanosheets, one efficient strategy is to construct 3D structures with hierarchical porous structures, good chemical/mechanical stabilities and tunable electrical conductivities. In this review, we firstly focus on the available synthetic approaches of 3D structures from 2D nanosheets, and then summarize the relationships between the microstructures of 3D structures built from 2D nanosheets and their electrochemical behaviors for lithium storage. On the basis of above results, some challenges are briefly discussed in the perspective of the development of various functional 3D structures.

关键词: Nanosheets, Atomic layers, Graphene, Three-dimensional structures, Lithium ion batteries

Abstract: 2D nanosheets such as graphene, silicene, phosphorene, metal dichalcogenides and MXenes are emerging and promising for lithium storage due to their ultrathin nature and corresponding chemical/physical properties. However, the serious restacking and aggregation of the 2D nanosheets are still hampering their applications. To circumvent the issues of 2D nanosheets, one efficient strategy is to construct 3D structures with hierarchical porous structures, good chemical/mechanical stabilities and tunable electrical conductivities. In this review, we firstly focus on the available synthetic approaches of 3D structures from 2D nanosheets, and then summarize the relationships between the microstructures of 3D structures built from 2D nanosheets and their electrochemical behaviors for lithium storage. On the basis of above results, some challenges are briefly discussed in the perspective of the development of various functional 3D structures.

Key words: Nanosheets, Atomic layers, Graphene, Three-dimensional structures, Lithium ion batteries