Two-dimensional organic cathode materials for alkali-metal-ion batteries

doi:10.1016/j.jechem.2017.11.008

能源化学(英文) ›› 2018, Vol. 27 ›› Issue (1): 86-98.DOI: 10.1016/j.jechem.2017.11.008

Two-dimensional organic cathode materials for alkali-metal-ion batteries

Chao Zhang^a, Chenbao Lu^a, Fan Zhang^a, Feng Qiu^b, Xiaodong Zhuang^a, Xinliang Feng^c

a Shanghai Key Lab of Electrical Insulation and Thermal Ageing, Shanghai Electrochemical Energy Devices Research Center, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, China;
b School of Chemical and Environmental Engineering, Shanghai Institute of Technology, Shanghai 201418, China;
c Department of Chemistry and Food Chemistry, Center for Advancing Electronics Dresden(cfaed), Technische Universität Dresden, 01062 Dresden, Germany

收稿日期:2017-10-31 修回日期:2017-11-02 出版日期:2018-01-15 发布日期:2018-01-13
通讯作者: Xiaodong Zhuang, Xinliang Feng
作者简介:Chao Zhang received his B.S. degree from Hefei University of Technology in June 2015;Chenbao Lu received his B.S. degree in Chemical Engineering and Technology from Nanjing University of Technology in June 2014 and received master's degree from Shanghai Jiao Tong University in March 2017; Fan Zhang received his B.Eng. degree in electrochemistry from Shanghai Jiao Tong University in 1991, and his Ph.D. in organic chemistry from Jilin University in 2000.
基金资助:
The authors thank the financial support from the 973 Programs of China (2013CBA01602), NSFC for Excellent Youth Scholars (51722304), NSFC (21720102002, 21574080 and 61306018), Shanghai Committee of Science and Technology (15JC1490500, 16JC1400703), and Open Project Program of the State Key Laboratory of Supramolecular Structure and Materials (sklssm201732, Jilin University); State Key Laboratory of Inorganic Synthesis and Preparative Chemistry (2016-08, Jilin University); State Key Laboratory for Mechanical Behavior of Materials (20161803, Xi'an Jiaotong University).

Two-dimensional organic cathode materials for alkali-metal-ion batteries

Chao Zhang^a, Chenbao Lu^a, Fan Zhang^a, Feng Qiu^b, Xiaodong Zhuang^a, Xinliang Feng^c

a Shanghai Key Lab of Electrical Insulation and Thermal Ageing, Shanghai Electrochemical Energy Devices Research Center, School of Chemistry and Chemical Engineering, Shanghai Jiao Tong University, Shanghai 200240, China;
b School of Chemical and Environmental Engineering, Shanghai Institute of Technology, Shanghai 201418, China;
c Department of Chemistry and Food Chemistry, Center for Advancing Electronics Dresden(cfaed), Technische Universität Dresden, 01062 Dresden, Germany

Received:2017-10-31 Revised:2017-11-02 Online:2018-01-15 Published:2018-01-13
Contact: Xiaodong Zhuang, Xinliang Feng
Supported by:
The authors thank the financial support from the 973 Programs of China (2013CBA01602), NSFC for Excellent Youth Scholars (51722304), NSFC (21720102002, 21574080 and 61306018), Shanghai Committee of Science and Technology (15JC1490500, 16JC1400703), and Open Project Program of the State Key Laboratory of Supramolecular Structure and Materials (sklssm201732, Jilin University); State Key Laboratory of Inorganic Synthesis and Preparative Chemistry (2016-08, Jilin University); State Key Laboratory for Mechanical Behavior of Materials (20161803, Xi'an Jiaotong University).

摘要/Abstract

摘要： With the increasing demand for large-scale battery systems in electric vehicles (EVs) and smart renewable energy grids, organic materials including small molecules and polymers utilized as electrodes in rechargeable batteries have received increasing attraction. In recent years, two-dimensional (2D) organic materials possessing planar layered architecture exhibit optional chemical modification, high specific surface area as well as unique electrical/magnetic properties, which have been emerging as the promising functional materials for wide applications in optoelectronics, catalysis, sensing, etc. Integrating with high-density redox-active sites and hierarchical porous structure, significant achievements in 2D organic materials as cathode materials for alkali-metal-ion batteries have been witnessed. In this review, the recent progress in synthetic approaches, structure analyses, electrochemical characterizations of 2D organic materials as well as their application in alkali-metal-ion batteries containing lithium ion battery (LIB), lithium sulfur battery (LSB), lithium air battery (LAB) and sodium ion battery (SIB) are summarized systematically, and their current challenges including cycling stability and electron conductivity for cathode materials in battery fields are also discussed.

关键词: Organic material, Two-dimensional, Cathode, Alkali-metal-ion battery

Abstract: With the increasing demand for large-scale battery systems in electric vehicles (EVs) and smart renewable energy grids, organic materials including small molecules and polymers utilized as electrodes in rechargeable batteries have received increasing attraction. In recent years, two-dimensional (2D) organic materials possessing planar layered architecture exhibit optional chemical modification, high specific surface area as well as unique electrical/magnetic properties, which have been emerging as the promising functional materials for wide applications in optoelectronics, catalysis, sensing, etc. Integrating with high-density redox-active sites and hierarchical porous structure, significant achievements in 2D organic materials as cathode materials for alkali-metal-ion batteries have been witnessed. In this review, the recent progress in synthetic approaches, structure analyses, electrochemical characterizations of 2D organic materials as well as their application in alkali-metal-ion batteries containing lithium ion battery (LIB), lithium sulfur battery (LSB), lithium air battery (LAB) and sodium ion battery (SIB) are summarized systematically, and their current challenges including cycling stability and electron conductivity for cathode materials in battery fields are also discussed.

Key words: Organic material, Two-dimensional, Cathode, Alkali-metal-ion battery

Chao Zhang, Chenbao Lu, Fan Zhang, Feng Qiu, Xiaodong Zhuang, Xinliang Feng. Two-dimensional organic cathode materials for alkali-metal-ion batteries[J]. 能源化学(英文), 2018, 27(1): 86-98.

Chao Zhang, Chenbao Lu, Fan Zhang, Feng Qiu, Xiaodong Zhuang, Xinliang Feng. Two-dimensional organic cathode materials for alkali-metal-ion batteries[J]. Journal of Energy Chemistry, 2018, 27(1): 86-98.

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Two-dimensional organic cathode materials for alkali-metal-ion batteries

Two-dimensional organic cathode materials for alkali-metal-ion batteries

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