Carbon-based derivatives from metal-organic frameworks as cathode hosts for Li-S batteries

doi:10.1016/j.jechem.2019.01.005

能源化学(英文版) ›› 2019, Vol. 38 ›› Issue (11): 94-113.DOI: 10.1016/j.jechem.2019.01.005

Carbon-based derivatives from metal-organic frameworks as cathode hosts for Li-S batteries

Qingping Wu^a,b, Xuejun Zhou^b, Jun Xu^a, Fahai Cao^a, Chilin Li^b

a State Key Laboratory of Chemical Engineering, East China University of Science and Technology, Shanghai 200237, China;
b State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, China

收稿日期:2018-12-16 修回日期:2019-01-03 出版日期:2019-11-15 发布日期:2020-12-18
通讯作者: Fahai Cao, fhcao@ecust.edu.cn; Chilin Li, chilinli@mail.sic.ac.cn
基金资助:
This work was partially supported by the Natural Science Foundation of China (No.11574111 to X-F.W.) and JSPS KAKENHI Grant Number JP16K05826 in Scientific Research (C) (to S.S.). This work was also supported by the Natural Science Foundation of Jilin Province (No. 20160101303JC, 20180101238JC, 20170204076GX, 20180101006JC to C.S.) and Post-Doctoral Innovative Talent Support Program (BX20180127 to S.W.).

Carbon-based derivatives from metal-organic frameworks as cathode hosts for Li-S batteries

Qingping Wu^a,b, Xuejun Zhou^b, Jun Xu^a, Fahai Cao^a, Chilin Li^b

a State Key Laboratory of Chemical Engineering, East China University of Science and Technology, Shanghai 200237, China;
b State Key Laboratory of High Performance Ceramics and Superfine Microstructure, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050, China

Received:2018-12-16 Revised:2019-01-03 Online:2019-11-15 Published:2020-12-18
Contact: Fahai Cao, fhcao@ecust.edu.cn; Chilin Li, chilinli@mail.sic.ac.cn
Supported by:
This work was partially supported by the Natural Science Foundation of China (No.11574111 to X-F.W.) and JSPS KAKENHI Grant Number JP16K05826 in Scientific Research (C) (to S.S.). This work was also supported by the Natural Science Foundation of Jilin Province (No. 20160101303JC, 20180101238JC, 20170204076GX, 20180101006JC to C.S.) and Post-Doctoral Innovative Talent Support Program (BX20180127 to S.W.).

摘要/Abstract

摘要： Lithium-sulfur batteries (Li-S batteries) are promising candidates for the next generation high-energy rechargeable Li batteries due to their high theoretical specific capacity (1672 mAh g^-1) and energy density (2500 Wh kg^-1). The commercialization of Li-S batteries is impeded by several key challenges at cathode side, e.g. the insulating nature of sulfur and discharged products (Li₂S₂ and Li₂S), the solubility of long-chain polysulfides and volume variation of sulfur cathode upon cycling. Recently, the carbonbased derivatives from metal-organic frameworks (MOFs) has emerged talent in their utilization as cathode hosts for Li-S batteries. They are not only highly conductive and porous to enable the acceleration of Li⁺/e^- transfer and accommodation of volumetric expansion of sulfur cathode during cycling, but also enriched by controllable chemical active sites to enable the adsorption of polysulfides and promotion of their conversion reaction kinetics. In this review, based on the types of MOFs (e.g. ZIF-8, ZIF-67, Prussian blue, Al-MOF, MOF-5, Cu-MOF, Ni-MOF), the synthetic methods, formation process and morphology, structural superiority of MOFs-derived carbon frameworks along with their electrochemical performance as cathode host in Li-S batteries are summarized and discussed.

关键词: Lithium-sulfur batteries, Carbon-based derivatives, Metal-organic frameworks, Cathode host

Abstract: Lithium-sulfur batteries (Li-S batteries) are promising candidates for the next generation high-energy rechargeable Li batteries due to their high theoretical specific capacity (1672 mAh g^-1) and energy density (2500 Wh kg^-1). The commercialization of Li-S batteries is impeded by several key challenges at cathode side, e.g. the insulating nature of sulfur and discharged products (Li₂S₂ and Li₂S), the solubility of long-chain polysulfides and volume variation of sulfur cathode upon cycling. Recently, the carbonbased derivatives from metal-organic frameworks (MOFs) has emerged talent in their utilization as cathode hosts for Li-S batteries. They are not only highly conductive and porous to enable the acceleration of Li⁺/e^- transfer and accommodation of volumetric expansion of sulfur cathode during cycling, but also enriched by controllable chemical active sites to enable the adsorption of polysulfides and promotion of their conversion reaction kinetics. In this review, based on the types of MOFs (e.g. ZIF-8, ZIF-67, Prussian blue, Al-MOF, MOF-5, Cu-MOF, Ni-MOF), the synthetic methods, formation process and morphology, structural superiority of MOFs-derived carbon frameworks along with their electrochemical performance as cathode host in Li-S batteries are summarized and discussed.

Key words: Lithium-sulfur batteries, Carbon-based derivatives, Metal-organic frameworks, Cathode host

Qingping Wu, Xuejun Zhou, Jun Xu, Fahai Cao, Chilin Li. Carbon-based derivatives from metal-organic frameworks as cathode hosts for Li-S batteries[J]. 能源化学(英文版), 2019, 38(11): 94-113.

Qingping Wu, Xuejun Zhou, Jun Xu, Fahai Cao, Chilin Li. Carbon-based derivatives from metal-organic frameworks as cathode hosts for Li-S batteries[J]. Journal of Energy Chemistry, 2019, 38(11): 94-113.

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Carbon-based derivatives from metal-organic frameworks as cathode hosts for Li-S batteries

Carbon-based derivatives from metal-organic frameworks as cathode hosts for Li-S batteries

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