Three dimensional porous frameworks for lithium dendrite suppression

doi:10.1016/j.jechem.2019.09.031

能源化学(英文版) ›› 2020, Vol. 44 ›› Issue (5): 73-89.DOI: 10.1016/j.jechem.2019.09.031

Three dimensional porous frameworks for lithium dendrite suppression

Shuyan Ni, Shuangshuang Tan, Qinyou An, Liqiang Mai

State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, Hubei, China

收稿日期:2019-05-17 修回日期:2019-09-18 出版日期:2020-05-15 发布日期:2020-12-18
基金资助:
This work was supported by the National Natural Science Foundation of China (51521001, 51832004 and 51602239), the National Natural Science Fund for Distinguished Young Scholars (51425204), and the Programme of Introducing Talents of Discipline to Universities (B17034), the Yellow Crane Talent (Science & Technology) Program of Wuhan City.

Three dimensional porous frameworks for lithium dendrite suppression

Shuyan Ni, Shuangshuang Tan, Qinyou An, Liqiang Mai

State Key Laboratory of Advanced Technology for Materials Synthesis and Processing, Wuhan University of Technology, Wuhan 430070, Hubei, China

Received:2019-05-17 Revised:2019-09-18 Online:2020-05-15 Published:2020-12-18
Contact: Qinyou An, Liqiang Mai
Supported by:
This work was supported by the National Natural Science Foundation of China (51521001, 51832004 and 51602239), the National Natural Science Fund for Distinguished Young Scholars (51425204), and the Programme of Introducing Talents of Discipline to Universities (B17034), the Yellow Crane Talent (Science & Technology) Program of Wuhan City.

摘要/Abstract

摘要： Lithium metal is a promising anode material owing to its very low electrochemical potential and ultrahigh specific capacity. However, the growth of lithium dendrites could result in a short lifespan, low coulombic efficiency, and potential safety hazards during the progress of lithium plating/stripping. These factors drastically hinder its application in lithium metal batteries. This review focuses on the use of three dimensional (3D) porous host frameworks to improve Li plating/stripping behaviors, accommodate the change in volume, and suppress or block lithium dendrite growth. Various 3D porous frameworks, including the conductive carbon-based, metal-based, and lithiophilic inorganic-compound frameworks are introduced and summarized in detail. The particular functions, relative developments, and optimized strategies of various 3D porous frameworks for lithium deposition/dissolution behaviors are discussed. Moreover, the challenges and promising developments in the field of Li metal anodes will be discussed at the end of this review.

关键词: Lithium metal battery, 3D porous frameworks, Lithium dendrite, Lithium sulfur batteries, Lithium oxygen batteries, Li plating/stripping

Abstract: Lithium metal is a promising anode material owing to its very low electrochemical potential and ultrahigh specific capacity. However, the growth of lithium dendrites could result in a short lifespan, low coulombic efficiency, and potential safety hazards during the progress of lithium plating/stripping. These factors drastically hinder its application in lithium metal batteries. This review focuses on the use of three dimensional (3D) porous host frameworks to improve Li plating/stripping behaviors, accommodate the change in volume, and suppress or block lithium dendrite growth. Various 3D porous frameworks, including the conductive carbon-based, metal-based, and lithiophilic inorganic-compound frameworks are introduced and summarized in detail. The particular functions, relative developments, and optimized strategies of various 3D porous frameworks for lithium deposition/dissolution behaviors are discussed. Moreover, the challenges and promising developments in the field of Li metal anodes will be discussed at the end of this review.

Key words: Lithium metal battery, 3D porous frameworks, Lithium dendrite, Lithium sulfur batteries, Lithium oxygen batteries, Li plating/stripping

Shuyan Ni, Shuangshuang Tan, Qinyou An, Liqiang Mai. Three dimensional porous frameworks for lithium dendrite suppression[J]. 能源化学(英文版), 2020, 44(5): 73-89.

Shuyan Ni, Shuangshuang Tan, Qinyou An, Liqiang Mai. Three dimensional porous frameworks for lithium dendrite suppression[J]. Journal of Energy Chemistry, 2020, 44(5): 73-89.

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Three dimensional porous frameworks for lithium dendrite suppression

Three dimensional porous frameworks for lithium dendrite suppression

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