Journal of Energy Chemistry ›› 2023, Vol. 79 ›› Issue (4): 37-44.DOI: 10.1016/j.jechem.2022.12.035

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Data-driven short circuit resistance estimation in battery safety issues

Yikai Jiaa,b, Jun Xua,b,c,*   

  1. aDepartment of Mechanical Engineering and Engineering Science, The University of North Carolina at Charlotte, Charlotte, NC 28223, USA;
    bVehicle Energy & Safety Laboratory (VESL), North Carolina Battery Complexity, Autonomous Vehicle and Electrification (BATT CAVE) Research Center, The University of North Carolina at Charlotte, Charlotte, NC 28223, USA;
    cSchool of Data Science, The University of North Carolina at Charlotte, Charlotte, NC 28223, USA
  • Received:2022-11-06 Revised:2022-12-05 Accepted:2022-12-14 Online:2023-04-15 Published:2023-05-30
  • Contact: * E-mail address: jun.xu@uncc.edu (J. Xu).

Abstract: Developing precise and fast methods for short circuit detection is crucial for preventing or mitigating the risk of safety issues of lithium-ion batteries (LIBs). In this paper, we developed a Convolutional Neural Networks (CNN) based model that can quickly and precisely predict the short circuit resistance of LIB cells during various working conditions. Cycling tests of cells with an external short circuit (ESC) are pro-duced to obtain the database and generate the training/ testing samples. The samples are sequences of voltage, current, charging capacity, charging energy, total charging capacity, total charging energy with a length of 120 s and frequency of 1 Hz, and their corresponding short circuit resistances. A big database with ~6 × 105 samples are generated, covering various short circuit resistances (47 ~ 470 X), current loading modes (Constant current-constant voltage (CC-CV) and drive cycle), and electrochemical states (cycle numbers from 1 to 300). Results show that the average relative absolute error of five random sam-ple splits is 6.75 %±2.8 %. Further parametric analysis indicates the accuracy estimation benefits from the appropriate model setups: the optimized input sequence length (~120 s), feature selection (at least one total capacity-related variable), and rational model design, using multiple layers with different kernel sizes. This work highlights the capabilities of machine learning algorithms and data-driven methodolo-gies in real-time safety risk prediction for batteries.

Key words: Lithium-ion battery, Safety risk, Internal short circuit, Short circuit resistance, Convolutional neural networks