Centimeter-sized Cs3Cu2I5 single crystals grown by oleic acid assisted inverse temperature crystallization strategy and their films for high- quality X-ray imaging

doi:10.1016/j.jechem.2022.12.016

Abstract

Abstract: Low-dimensional halide perovskites have become the most promising candidates for X-ray imaging, yet the issues of the poor chemical stability of hybrid halide perovskite, the high poisonousness of lead halides and the relatively low detectivity of the lead-free halide perovskites which seriously restrain its commercialization. Here, we developed a solution inverse temperature crystal growth (ITCG) method to bring-up high quality Cs₃Cu₂I₅ crystals with large size of centimeter order, in which the oleic acid (OA) is introduced as an antioxidative ligand to inhibit the oxidation of cuprous ions effieiently, as well as to decelerate the crystallization rate remarkalby. Based on these fine crystals, the vapor deposition tech-nique is empolyed to prepare high quality Cs₃Cu₂I₅ films for efficient X-ray imaging. Smooth surface mor-phology, high light yields and short decay time endow the Cs₃Cu₂I₅ films with strong radioluminescence, high resolution (12 lp/mm), low detection limits (53 nGy_air/s) and desirable stability. Subsequently, the Cs₃Cu₂I₅ films have been applied to the practical radiography which exhibit superior X-ray imaging per-formance. Our work provides a paradigm to fabricate nonpoisonous and chemically stable inorganic halide perovskite for X-ray imaging.

Key words: Inverse temperature crystal growth, Cs₃Cu₂I₅ single crystal, Vapor deposition, Cs₃Cu₂I₅ films, X-ray imaging

Tao Chen, Xin Li, Yong Wang, Feng Lin, Ruliang Liu, Wenhua Zhang, Jie Yang, Rongfei Wang, Xiaoming Wen, Bin Meng, Xuhui Xu, Chong Wang. Centimeter-sized Cs₃Cu₂I₅ single crystals grown by oleic acid assisted inverse temperature crystallization strategy and their films for high- quality X-ray imaging[J]. Journal of Energy Chemistry, 2023, 79(4): 382-389.

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URL: https://www.jenergychem.com/EN/10.1016/j.jechem.2022.12.016

https://www.jenergychem.com/EN/Y2023/V79/I4/382

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Centimeter-sized Cs₃Cu₂I₅ single crystals grown by oleic acid assisted inverse temperature crystallization strategy and their films for high- quality X-ray imaging

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