Enhanced rate and specific capacity in nanorod-like core-shell crystalline NiMoO4@amorphous cobalt boride materials enabled by Mott-Schottky heterostructure as positive electrode for hybrid supercapacitors

doi:10.1016/j.jechem.2023.06.023

Abstract

Abstract: The supercapacitor electrode materials suffer from structure pulverization and sluggish electrode kinetics under high current rates. Herein, a unique NiMoO₄@Co-B heterostructure composed of highly conductive Co-B nanoflakes and a semiconductive NiMoO₄ nanorod is designed as an electrode material to exert the energy storage effect on supercapacitors. The formed Mott-Schottky heterostructure is helpful to overcome the ion diffusion barrier and charge transfer resistance during charging and discharging. Moreover, this crystalline-amorphous heterogeneous phase could provide additional ion storage sites and better strain adaptability. Remarkably, the optimized NiMoO₄@Co-B hierarchical nanorods (the mass ratio of NiMoO₄/Co-B is 3:1) present greatly enhanced electrochemical characteristics compared with other components, and show superior specific capacity of 236.2 mA h g^-1 at the current density of 0.5 A g^-1, as well as remarked rate capability. The present work broadens the horizons of advanced electrode design with distinct heterogeneous interface in other energy storage and conversion field.

Key words: Crystalline-amorphous heterophase, Mott-Schottky heterostructure, Energy storage, Nickel molybdate

Jing-Feng Hou, Jian-Fei Gao, Ling-Bin Kong. Enhanced rate and specific capacity in nanorod-like core-shell crystalline NiMoO₄@amorphous cobalt boride materials enabled by Mott-Schottky heterostructure as positive electrode for hybrid supercapacitors[J]. Journal of Energy Chemistry, 2023, 85(10): 276-287.

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URL: https://www.jenergychem.com/EN/10.1016/j.jechem.2023.06.023

https://www.jenergychem.com/EN/Y2023/V85/I10/276

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Enhanced rate and specific capacity in nanorod-like core-shell crystalline NiMoO₄@amorphous cobalt boride materials enabled by Mott-Schottky heterostructure as positive electrode for hybrid supercapacitors

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