Recent progress and challenges in structural construction strategy of metal-based catalysts for nitrate electroreduction to ammonia

doi:10.1016/j.jechem.2023.07.006

Abstract

Abstract: Ammonia plays an essential role in human production and life as a raw material for chemical fertilizers. The nitrate electroreduction to ammonia reaction (NO₃RR) has garnered attention due to its advantages over the Haber-Bosch process and electrochemical nitrogen reduction reaction. Therefore, it represents a promising approach to safeguard the ecological environment by enabling the cycling of nitrogen species. This review begins by discussing the theoretical insights of the NO₃RR. It then summarizes recent advances in catalyst design and construction strategies, including alloying, structure engineering, surface engineering, and heterostructure engineering. Finally, the challenges and prospects in this field are presented. This review aims to guide for enhancing the efficiency of electrocatalysts in the NO₃RR, and offers insights for converting NO₃^- to NH₃.

Key words: Nitrate electroreduction to ammonia reaction (NO₃RR), Structural construction strategy, Nitrogen cycle, Metal-based catalysts, Catalytic mechanism

Shuai Niu. Recent progress and challenges in structural construction strategy of metal-based catalysts for nitrate electroreduction to ammonia[J]. Journal of Energy Chemistry, 2023, 86(11): 69-83.

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References

[1] E. Boyle, Science 356 (2017) 700-701.
[2] D.E. Canfield, A.N. Glazer, P.G. Falkowski, Science 330 (2010) 192-196.
[3] V. Rosca, M. Duca, M.T.de Groot, M.T.M. Koper, Chem. Rev. 109(2009) 2209-2244.
[4] M. Duca, M.T.M.Koper, Energy Environ. Sci. 5(2012) 9726-9742.
[5] J.N. Galloway, A.R. Townsend, J.W. Erisman, M. Bekunda, Z. Cai, J.R. Freney, L. A. Martinelli, S.P. Seitzinger, M.A. Sutton, Science 320 (2008) 889-892.
[6] J.G. Chen, R.M. Crooks, L.C. Seefeldt, K.L. Bren, R.M. Bullock, M.Y. Darensbourg, P.L. Holland, B. Hoffman, M.J. Janik, A.K. Jones, M.G. Kanatzidis, P. King, K.M. Lancaster, S.V. Lymar, P. Pfromm, W.F. Schneider, R.R. Schrock, Science 360 (2018) eaar6611.
[7] J. Martínez, A. Ortiz, I. Ortiz, Appl. Catal., B 207 (2017) 42-59.
[8] H.O.N.Tugaoen, S. Garcia-Segura, K.Hristovski, P. Westerhoff, Sci. Total Environ. 599-600(2017) 1524-1551.
[9] X. Zhang, Y. Wang, C. Liu, Y. Yu, S. Lu, B. Zhang,Chem. Eng. J. 403(2021).
[10] Y. Zeng, C. Priest, G. Wang, G. Wu, Small Methods 4 (2020) 2000672.
[11] M. Alikhani, M.R. Moghbeli, Chem. Eng. J. 239(2014) 93-104.
[12] S. Samatya, N. Kabay, Ü. Yüksel, M. Arda, M. Yüksel, React. Funct. Polym. 66(2006) 1206-1214.
[13] L.J. Banasiak, A.I. Schäfer, J. Membr. Sci. 334(2009) 101-109.
[14] D. Xu, Y. Li, L. Yin, Y. Ji, J. Niu, Y. Yu, Front. Environ. Sci. Eng. 12(2018) 9.
[15] R. Epsztein, O. Nir, O. Lahav, M. Green, Chem. Eng. J. 279(2015) 372-378.
[16] N. Barrabés, J. Sá, Appl. Catal., B 104 (2011) 1-5.
[17] F. Djouadi Belkada, O. Kitous, N. Drouiche, S. Aoudj, O. Bouchelaghem, N. Abdi, H. Grib, N. Mameri, Sep. Purif. Technol. 204(2018) 108-115.
[18] L. Jelínek, H. Parschová, Z. Matĕjka, M. Paidar, K. Bouzek, Water Environ. Res 76 (2004) 2686-2690.
[19] P.H. van Langevelde, I. Katsounaros, M.T.M. Koper, Joule 5 (2021) 290-294.
[20] Y. Wang, Y. Yu, R. Jia, C. Zhang, B. Zhang, Natl. Sci. Rev. 6(2019) 730-738.
[21] S. Guo, K. Heck, S. Kasiraju, H. Qian, Z. Zhao, L.C. Grabow, J.T. Miller, M.S. Wong, ACS Catal. 8(2018) 503-515.
[22] L. Sun, B. Liu, Adv. Mater. 35(2023) 2207305.
[23] H. Zou, W. Rong, S. Wei, Y. Ji, L. Duan, Proc. Natl. Acad. Sci. 117(2020) 29462-29468.
[24] C. Tang, S.-Z.Qiao, Chem. Soc. Rev. 48(2019) 3166-3180.
[25] S.Z. Andersen, V. Čolić, S. Yang, J.A. Schwalbe, A.C. Nielander, J.M. McEnaney, K. Enemark-Rasmussen, J.G. Baker, A.R. Singh, B.A. Rohr, M.J. Statt, S.J. Blair, S. Mezzavilla, J. Kibsgaard, P.C.K. Vesborg, M. Cargnello, S.F. Bent, T.F. Jaramillo, I.E.L. Stephens, J.K. Nørskov, I. Chorkendorff, Nature 570 (2019) 504-508.
[26] B.P. Dash, S. Chaudhari, Water Res. 39(2005) 4065-4072.
[27] A.S. Bandarenka, M.T.M.Koper, J. Catal. 308(2013) 11-24.
[28] F. Lv, M. Sun, Y. Hu, J. Xu, W. Huang, N. Han, B. Huang, Y. Li, Energy Environ. Sci. 16(2023) 201-209.
[29] J.-Y.Fang, Q.-Z. Zheng, Y.-Y. Lou, K.-M. Zhao, S.-N. Hu, G. Li, O. Akdim, X.-Y. Huang, S.-G. Sun, Nat. Commun. 13(2022) 7899.
[30] L. Niu, L. An, X. Wang, Z. Sun, J. Energy Chem. 61(2021) 304-318.
[31] M. Li, H. Huang, J. Low, C. Gao, R. Long, Y. Xiong, Small Methods 3 (2019) 1800388.
[32] S. Taguchi, J.M. Feliu, Electrochim. Acta 52 (2007) 6023-6033.
[33] M. Duca, M.O. Cucarella, P. Rodriguez, M.T.M.Koper, J. Am. Chem. Soc. 132(2010) 18042-18044.
[34] J. Yang, P. Sebastian, M. Duca, T. Hoogenboom, M.T.M.Koper, Chem. Commun. 50(2014) 2148-2151.
[35] D. Chen, S. Zhang, D. Yin, W. Li, X. Bu, Q. Quan, Z. Lai, W. Wang, Y. Meng, C. Liu, S. Yip, F.-R.Chen, C. Zhi, J.C. Ho, Adv. Energy Mater. 13(2023) 2203201.
[36] J. Lim, C.-Y.Liu, J. Park, Y.-H. Liu, T.P. Senftle, S.W. Lee, M.C. Hatzell, ACS Catal. 11(2021) 7568-7577.
[37] X. Wang, M. Zhu, G. Zeng, X. Liu, C. Fang, C. Li, Nanoscale 12 (2020) 9385-9391.
[38] N.C. Kani, N.H.L.Nguyen, K. Markel, R.R. Bhawnani, B. Shindel, K. Sharma, S. Kim, V.P. Dravid, V. Berry, J.A. Gauthier, M.R. Singh, Adv. Energy Mater. 13(2023) 2204236.
[39] J. Wang, Y. Wang, C. Cai, Y. Liu, D. Wu, M. Wang, M. Li, X. Wei, M. Shao, M. Gu, Nano Lett. 23(2023) 1897-1903.
[40] S. Zhang, M. Li, J. Li, Q. Song, X. Liu, Proc. Natl. Acad. Sci. 120(2023) e2207080119.
[41] Z. Xi, J. Wang, B. Liu, X. Xu, P. Jing, R. Gao, J. Zhang, J. Energy Chem. 83(2023) 32-42.
[42] Q. Gao, B. Yao, H.S. Pillai, W. Zang, X. Han, Y. Liu, S.-W. Yu, Z. Yan, B. Min, S. Zhang, H. Zhou, L. Ma, H. Xin, Q. He, H. Zhu, Nat. Synth. (2023), https://doi.org/10.1038/s44160-023-00258-x.
[43] Z. Wang, S.D. Young, B.R. Goldsmith, N. Singh, J. Catal. 395(2021) 143-154.
[44] J.-X.Liu, D. Richards, N. Singh, B.R. Goldsmith, ACS Catal. 9(2019) 7052-7064.
[45] M.T.de Groot, M.T.M. Koper, J. Electroanal. Chem. 562(2004) 81-94.
[46] S. Garcia-Segura, M. Lanzarini-Lopes, K. Hristovski, P. Westerhoff, Appl. Catal., B 236 (2018) 546-568.
[47] A.C.A. de Vooys, R.A.van Santen, J.A.R.van Veen, J. Mol. Catal. A: Chem. 154(2000) 203-215.
[48] G.E. Dima, A.C.A.de Vooys, M.T.M. Koper, J. Electroanal. Chem. 554-555(2003) 15-23.
[49] J. Long, S. Chen, Y. Zhang, C. Guo, X. Fu, D. Deng, J. Xiao, Angew. Chem. Int. Ed. 59(2020) 9711-9718.
[50] A.C.A. de Vooys, M.T.M. Koper, R.A.van Santen, J.A.R.van Veen, J. Catal. 202(2001) 387-394.
[51] A. Vooys, G. Beltramo, B. Van Riet, J. Van Veen, M. Koper, Electrochim. Acta 49 (2004) 1307-1314.
[52] J. Yang, M. Duca, K.J.P.Schouten, M.T. Koper, J. Electroanal. Chem. 662(2011) 87-92.
[53] R. Zhang, D. Shuai, K.A. Guy, J.R. Shapley, T.J. Strathmann, C.J. Werth, ChemCatChem 5 (2013) 313-321.
[54] J. Gao, B. Jiang, C. Ni, Y. Qi, Y. Zhang, N. Oturan, M.A. Oturan, Appl. Catal., B 254 (2019) 391-402.
[55] J. Gao, B. Jiang, C. Ni, Y. Qi, X. Bi,Chem. Eng. J. 382(2020).
[56] H. Shin, S. Jung, S. Bae, W. Lee, H. Kim, Environ. Sci. Technol. 48(2014) 12768-12774.
[57] B.P. Chaplin, M. Reinhard, W.F. Schneider, C. Schüth, J.R. Shapley, T.J. Strathmann, C.J. Werth, Environ. Sci. Technol. 46(2012) 3655-3670.
[58] T. Hu, C. Wang, M. Wang, C.M. Li, C. Guo, ACS Catal. 11(2021) 14417-14427.
[59] X. Fu, X. Zhao, X. Hu, K. He, Y. Yu, T. Li, Q. Tu, X. Qian, Q. Yue, M.R. Wasielewski,Appl. Mater. Today 19(2020).
[60] Y. Xu, M. Wang, K. Ren, T. Ren, M. Liu, Z. Wang, X. Li, L. Wang, H. Wang, J. Mater. Chem. A 9 (2021) 16411-16417.
[61] H. Wang, Q. Mao, T. Ren, T. Zhou, K. Deng, Z. Wang, X. Li, Y. Xu, L. Wang, ACS Appl. Mater. Interfaces 13 (2021) 44733-44741.
[62] T. Zhu, Q. Chen, P. Liao, W. Duan, S. Liang, Z. Yan, C. Feng, Small 16 (2020) 2004526.
[63] Q. Wu, M. Luo, J. Han, W. Peng, Y. Zhao, D. Chen, M. Peng, J. Liu, F.M.F.de Groot, Y.Tan, ACS Energy Lett. 5(2020) 192-199.
[64] C. Gao, H. Wang, S. Li, B. Liu, J. Yang, J. Gao, Z. Peng, Z. Zhang, Z. Liu,Electrochim. Acta 327(2019).
[65] K. Li, Y. Li, Y. Wang, J. Ge, C. Liu, W. Xing, Energy Environ. Sci. 11(2018) 1232-1239.
[66] J. Chen, Y. Yang, J. Su, P. Jiang, G. Xia, Q. Chen, ACS Appl. Mater. Interfaces 9 (2017) 3596-3601.
[67] L. Bu, S. Guo, X. Zhang, X. Shen, D. Su, G. Lu, X. Zhu, J. Yao, J. Guo, X. Huang, Nat. Commun. 7(2016) 11850.
[68] J. Ding, L. Bu, S. Guo, Z. Zhao, E. Zhu, Y. Huang, X. Huang, Nano Lett. 16(2016) 2762-2767.
[69] W. Tong, B. Huang, P. Wang, L. Li, Q. Shao, X. Huang, Angew. Chem. Int. Ed. 132(2020) 2671-2675.
[70] R. Zhao, H. Xie, L. Chang, X. Zhang, X. Zhu, X. Tong, T. Wang, Y. Luo, P. Wei, Z. Wang, EnergyChem 1(2019).
[71] X. Li, P. Shen, Y. Luo, Y. Li, Y. Guo, H. Zhang, K. Chu, Angew. Chem. Int. Ed. 61(2022) e202205923.
[72] W. Luc, C. Collins, S. Wang, H. Xin, K. He, Y. Kang, F. Jiao, J. Am. Chem.Soc. 139(2017) 1885-1893.
[73] Y. Pi, Q. Shao, P. Wang, J. Guo, X. Huang, Adv. Funct. Mater. 27(2017) 1700886.
[74] J.T. Matsushima, V.C. Fernandes, A.B. Couto, M.R. Baldan, N.G. Ferreira,Int. J. Electrochem. 2012(2012).
[75] L. Mattarozzi, S. Cattarin, N. Comisso, P. Guerriero, M. Musiani, L. Vázquez-Gómez, E. Verlato, Electrochim. Acta 89 (2013) 488-496.
[76] Y. Wang, A. Xu, Z. Wang, L. Huang, J. Li, F. Li, J. Wicks, M. Luo, D.-H.Nam, C.-S. Tan, Y. Ding, J. Wu, Y. Lum, C.-T. Dinh, D. Sinton, G. Zheng, E.H. Sargent, J. Am. Chem. Soc. 142(2020) 5702-5708.
[77] Q. Gao, H.S. Pillai, Y. Huang, S. Liu, Q. Mu, X. Han, Z. Yan, H. Zhou, Q. He, H. Xin, H. Zhu, Nat. Commun. 13(2022) 2338.
[78] Y. Zhang, X. Chen, W. Wang, L. Yin, J.C. Crittenden,Appl. Catal., B 310(2022).
[79] S. Wang, L. Li, K.S. Hui, D.A. Dinh, Z. Lu, Q. Zhang, K.N. Hui, Nano Energy 113 (2023).
[80] J. Cai, Y. Wei, A. Cao, J. Huang, Z. Jiang, S. Lu, S.-Q. Zang, Appl. Catal., B 316(2022).
[81] K. Chen, Z. Ma, X. Li, J. Kang, D. Ma, K. Chu, Adv. Funct. Mater. 33(2023) 2209890.
[82] S. Li, P. Ma, C. Gao, L. Liu, X. Wang, M. Shakouri, R. Chernikov, K. Wang, D. Liu, R. Ma, Energy Environ. Sci. 15(2022) 3004-3014.
[83] J. Wang, C. Cai, Y. Wang, X. Yang, D. Wu, Y. Zhu, M. Li, M. Gu, M. Shao, ACS Catal. 11(2021) 15135-15140.
[84] J.-Y. Zhu, Q. Xue, Y.-Y. Xue, Y. Ding, F.-M. Li, P. Jin, P. Chen, Y. Chen, ACS Appl. Mater. Interfaces 12 (2020) 14064-14070.
[85] X. Deng, Y. Yang, L. Wang, X.Z. Fu, J.L. Luo, Adv. Sci. 8(2021) 2004523.
[86] S. Ye, Z. Chen, G. Zhang, W. Chen, C. Peng, X. Yang, L. Zheng, Y. Li, X. Ren, H. Cao, D. Xue, J. Qiu, Q. Zhang, J. Liu, Energy Environ. Sci. 15(2022) 760-770.
[87] R. Jia, Y. Wang, C. Wang, Y. Ling, Y. Yu, B. Zhang, ACS Catal. 10(2020) 3533-3540.
[88] W. Zhong, Z. Gong, Z. He, N. Zhang, X. Kang, X. Mao, Y. Chen, J. Energy Chem. 78(2023) 211-221.
[89] Y. Guo, R. Zhang, S. Zhang, Y. Zhao, Q. Yang, Z. Huang, B. Dong, C. Zhi, Energy Environ. Sci. 14(2021) 3938-3944.
[90] J. Li, G. Zhan, J. Yang, F. Quan, C. Mao, Y. Liu, B. Wang, F. Lei, L. Li, A.W.M.Chan, L. Xu, Y.Shi, Y. Du, W. Hao, P.K. Wong, J. Wang, S.-X. Dou, L. Zhang, J.C. Yu, J. Am. Chem. Soc. 142(2020) 7036-7046.
[91] Q. Hu, Y. Qin, X. Wang, Z. Wang, X. Huang, H. Zheng, K. Gao, H. Yang, P. Zhang, M. Shao, Energy Environ. Sci. 14(2021) 4989-4997.
[92] X. Fu, X. Zhao, X. Hu, K. He, Y. Yu, T. Li, Q. Tu, X. Qian, Q. Yue, M.R. Wasielewski, Y. Kang,Appl. Mater. Today 19(2020).
[93] Y. Han, X. Zhang, W. Cai, H. Zhao, Y. Zhang, Y. Sun, Z. Hu, S. Li, J. Lai, L. Wang, J. Colloid Interface Sci. 600(2021) 620-628.
[94] N. Zhang, G. Zhang, P. Shen, H. Zhang, D. Ma, K. Chu, Adv. Funct. Mater. 33(2023) 2211537.
[95] Y. Luo, K. Chen, G. Wang, G. Zhang, N. Zhang, K. Chu, Inorg. Chem. Front. 10(2023) 1543-1551.
[96] G. Wang, P. Shen, K. Chen, Y. Guo, X. Zhao, K. Chu, Inorg. Chem. Front. 10(2023) 2014-2021.
[97] Y. Fu, S. Wang, Y. Wang, P. Wei, J. Shao, T. Liu, G. Wang, X. Bao, Angew. Chem. Int. Ed. 62(2023) e202303327.
[98] Y. Wang, W. Zhou, R. Jia, Y. Yu, B. Zhang, Angew. Chem. Int. Ed. 59(2020) 5350-5354.
[99] J. Cai, S. Qin, M.A. Akram, X. Hou, P. Jin, F. Wang, B. Zhu, X. Li, L. Feng, J. Mater. Chem. A 10 (2022) 12669-12678.
[100] W.-J.Sun, H.-Q. Ji, L.-X. Li, H.-Y. Zhang, Z.-K. Wang, J.-H. He, J.-M. Lu, Angew. Chem. Int. Ed. 60(2021) 22933-22939.
[101] Y. Yu, C. Wang, Y. Yu, Y. Wang, B. Zhang, Sci. China Chem. 63(2020) 1469-1476.
[102] X. Li, P. Shen, X. Li, D. Ma, K. Chu, ACS Nano 17 (2023) 1081-1090.
[103] Y. Wang, C. Liu, B. Zhang, Y. Yu, Sci. China Mater 63 (2020) 2530-2538.
[104] Y. Cui, A. Dong, Y. Zhou, Y. Qu, M. Zhao, Z. Wang, Q. Jiang, Small 19 (2023) 2207661.
[105] T. Ren, K. Ren, M. Wang, M. Liu, Z. Wang, H. Wang, X. Li, L. Wang, Y. Xu,Chem. Eng. J. 426(2021).
[106] L. Su, K. Li, H. Zhang, M. Fan, D. Ying, T. Sun, Y. Wang, J. Jia, Water Res. 120(2017) 1-11.
[107] W. He, J. Zhang, S. Dieckhöfer, S. Varhade, A.C. Brix, A. Lielpetere, S. Seisel, J.R. C.Junqueira, W. Schuhmann, Nat. Commun. 13(2022) 1129.
[108] F. Liu, K. Liu, M. Li, S. Hu, J. Li, X. Lei, X. Liu, Chemosphere 223 (2019) 560-568.
[109] P. Li, R. Li, Y. Liu, M. Xie, Z. Jin, G. Yu, J. Am. Chem.Soc. 145(2023) 6471-6479.
[110] F.-Y.Chen, Z.-Y. Wu, S. Gupta, D.J. Rivera, S.V. Lambeets, S. Pecaut, J.Y.T. Kim, P. Zhu, Y.Z. Finfrock, D.M. Meira, G. King, G. Gao, W. Xu, D.A. Cullen, H. Zhou, Y. Han, D.E. Perea, C.L. Muhich, H. Wang, Nat. Nanotechnol. 17(2022) 759-767.
[111] G. Zhang, X. Li, K. Chen, Y. Guo, D. Ma, K. Chu, Angew. Chem. Int. Ed. 62(2023) e202300054.
[112] W. Gao, K. Xie, J. Xie, X. Wang, H. Zhang, S. Chen, H. Wang, Z. Li, C. Li, Adv. Mater. 35(2023) 2202952.
[113] Y. Wang, S. Shu, M. Peng, L. Hu, X. Lv, Y. Shen, H. Gong, G. Jiang, Nanoscale 13 (2021) 17504-17511.